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Picosecond Schrödinger cat states for ultrafast optical quantum processing

Mamoru Endo, Kan Takase, Takefumi Nomura, Tatsuki Sonoyama, Kazuma Takahashi, Sachiko Takasu, Daiji Fukuda, Takahiro Kashiwazaki, Asuka Inoue, Takeshi Umeki, Peter van Loock, Petr Marek, Radim Filip, Warit Asavanant, Akira Furusawa·June 22, 2026
Quantum Physicsphysics.optics

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Abstract

Non-Gaussian states are essential resources for universal, fault-tolerant optical quantum computing, but their generation rate remains limited by low heralding probabilities and operation in nanosecond temporal modes. Here, we demonstrate multi-photon generalized photon subtraction in picosecond optical wave packets, establishing the state-generation capability required for high-rate operation by addressing the temporal-mode bottleneck that has constrained the achievable rate. Two interfering ultrashort squeezed vacua are heralded by photon-number-resolving detection with a high-speed transition-edge sensor and characterized by pulsed homodyne detection matched to 10-ps temporal modes at a 5-MHz pump repetition rate. We reconstruct Wigner functions without loss correction that exhibit up to four distinct negative regions for four-photon heralding, together with an effective cat-state amplitude of $α_{\mathrm{eff}} = 1.69$. This amplitude approaches the range of practical relevance for fault-tolerant cat-code architectures and for adaptive breeding toward logical-qubit generation, while the picosecond temporal mode establishes a platform compatible with high-rate, scalable time-multiplexed photonic architectures.

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